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"+D=' = @B + 80@(    0(P 7    b*     0pP J e7 P d*     60P K  P b*     6 P J eK P d*   H  0 e彖 ? ̙3380___PPT10.h 0L0 0$(  r  S yw y r  S y   y H  0޽h ? 33___PPT10i.fy+D=' = @B +  0L0   0(   x  c $j   x  c $1H Pe  H  0޽h ? 33___PPT10i.fPب+D=' = @B + 0L0 Ph(     6l 'gt ~0MAJOR FACTORS INFLUENCING URBAN AIR POLLUTION /111"0    TA 13_08_2_web' -,$@  0   VA 13_07_20_webw g-,$@  0   0g Y  > 2   0|o TUrban sources of emission, temporal and spatial variation of their characteristics $U S$3$T   s *|"`',$D  0 x(Urban vehicular and industrial emissions)(2)( H  0޽h ? 33  ___PPT10y .f`O+7<oD ' i= @B D ' = @BA?%,( < +O%,( < +D ' =%(D ' =%(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<* %(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<* D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<* D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<* %(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<* D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<* D' =A@BBBB0B%(D' =1:Bvisible*o3>+B#style.visibility<*%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*+8+0+0 + 0L0 `J(    6|#   `} ~0MAJOR FACTORS INFLUENCING URBAN AIR POLLUTION /211"0   c 8A c8=310712'f,$@  0  0# qi z&Meteorological and synoptic conditions'(2'$3&   s *# "`,$D  0 Midday surface pressure and air temperature fields corresponding to the highest ozone concentrations in St. Petersburg in 2002, July 31 (weather map downloaded from the Kln University site) 2 H  0޽h ? 33  ___PPT10 .fCl+ܳ3DO ' p# = @B D ' = @BA?%,( < +O%,( < +DA' =%(D' =%(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*D' =A@BBBB0B%(D' =1:Bvisible*o3>+B#style.visibility<*%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*+8+0+0 + 0L0 LDp(    6#   `} ~0MAJOR FACTORS INFLUENCING URBAN AIR POLLUTION /311"0   c JA& chagall_nadgorodom}T ,$@  0  0G#  OStructure of the urban canopy, location, shape and size of buildings, roads etcP 2P$3O   0J# C ,$  0 mMarc Chagall "Above the city" 2 H  0޽h ? 33  ___PPT10 .f@1+dDO ' # = @B D ' = @BA?%,( < +O%,( < +DA' =%(D' =%(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*D' =A@BBBB0B%(D' =1:Bvisible*o3>+B#style.visibility<*%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*+8+0+0 + 0L0 ~v (     6Tc   `} x*URBAN AIR POLLUTION FORECASTS -- WHAT FOR?++"*   0f   ` DTo warn people about possible high-pollution episodes in the city; To provide information for policy- and decision-makers in order to implement emission-control measures, like emission reduction at stationary sources, limitations imposed on traffic intensity and pattern etc, resulting in reduction of peak concentrations EZED H  0޽h ? 33___PPT10i.f02x+D=' = @B + 0L0 $/(  $ $ 6yI   `} }/PROBLEMS WITH PREDICTION OF URBAN AIR POLLUTION00"/   $ 0d~  ` `Emission parameters and their temporal and spatial variability are not known well; Fields of mean and turbulent characteristics of the wind flow transporting pollutants are non-uniform and have sharp gradients; Concentration fields are highly irregular in space and time; Concentrations are excessively noisy (include intensive stochastic component); aa` H $ 0޽h ? 33___PPT10i.f+D=' = @B + 0L0 ,R(  ,' , B~ ?wq gStochastic component in atmospheric processes limiting precision of dispersion models and forecasts (1)hhg  , 0$~   qPlume meandering (PP ` , 0~    pF. Gifford (1958): Probability density of fluctuations of centerline concentrations due to the plume meandering:JP^P]p L    ,# S0  ," <A ?  ~  , C BXC DE4F| X 8(hpx8``HX0@( @    "`0  , HA  ?"6@ NNN?N` T H , 0޽h ? 33___PPT10i.fp"+D=' = @B +T 0L0 SK0(  0x 0 <A ??/Y ' 0 B41~ ?wq gStochastic component in atmospheric processes limiting precision of dispersion models and forecasts (2)hhg  0 0h5~ T, 8The straight line corresponds to the best lognormal fit ,9(288 H 0 0޽h ? 33___PPT10i.f{̈+D=' = @B + 0L0  42(  4 4 0l[    6Deterministic models can predict non-stochastic characteristics (conditional statistics) of atmospheric properties (e.g., math expectations, percentiles, PDFs, ensembles and so on); Comparison of predictions of a deterministic model with stochastic measurements results in errors that cannot be eliminated by any improvements and tuning of the model; Error of prediction at the plume axis is about 100% and at the fixed space/time point is of the order of 1000%.P.  0  4 0 K   ,$  0 }Mean square stochastic error in the axial GLC for a "perfect" dispersion model for a single point source (Genikhovich, 2003) 0}}} x V { | 4 6A ? ` |,$D  0'  4 B8L  ?wq gStochastic component in atmospheric processes limiting precision of dispersion models and forecasts (3)hhg H 4 0޽h ? 33  ___PPT10 .fv+eDO ' ~= @B D ' = @BA?%,( < +O%,( < +DA' =%(D' =%(D' =A@BBBB0B%(D' =1:Bvisible*o3>+B#style.visibility<*4}%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*4}D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*4}D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*4%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*4D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*4+8+0+40 +  0L0 80(  8x 8 c $ j   x 8 c $ Pe   H 8 0޽h ? 33___PPT10i.f d+D=' = @B +%/ 0L0 ?7((  ( ( 6<R  `< 1TWO MAIN APPROACHES TO AIR POLLUTION FORECASTING221  ( s *UR "`/ i,$@  0 Deterministic forecast Based on general physical principles and semi-empirical parameterizations; Very sensitive to errors in emission- and meteorological data; Cannot not reproduce the stochastic component of air pollution; Needs monitoring data only for validation purposes;0ZZ  ( s *R "`/m ]i,$@  0 iStatistical forecast Based on empirical relationships between characteristics of the air pollution ("predictants") and governing parameters ("predictors"); Doesn't make use of emission data; In principle, can reproduce all components of the turbulent spectra; Uses monitoring data for constructing and teaching the model as well as for its "initialization"; 0ZUZU.e    H ( 0޽h ? 33v(n(___PPT10N(.fӎ+DD"(' = @B D'' = @BA?%,( < +O%,( < +D' =%(D.' =%(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(c%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(cD' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(cD' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(c%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(cD' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(cD' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(D' =%(D.' =%(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(D' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(D' =4@BBBB%(D' =1:Bvisible*o3>+B#style.visibility<*(j%(D' =+4 8?\CB#ppt_xBCB#ppt_xB*Y3>B ppt_x<*(jD' =+4 8?dCB1+#ppt_h/2BCB#ppt_yB*Y3>B ppt_y<*(j+  0L0 @*(  @x @ c $H j  H  r @ S XH  H  H @ 0޽h ? 33___PPT10i.ff+D=' = @B + 0L0 j(  k  B<9R YPDF OF RATIOS OF MEASURED AROUND ALUMINUM PLANTS AND CALCULATED MAJORANT CONCENTRATIONS T2( 1" &"   (1 & <  3 A?3w  009 #  Measured concentrations are less than 1.25 times calculated ones in 98% of all observations. Thus, the field of the 98th percentiles is calculated with the error of 25%.> 2v 2    s *9"`v] BThis PDF was estimated using ~50,000 measured concentrations of HFC 2CB H  0޽h ? 33___PPT10i.&g@R&+D=' = @B +[ 0L0 ZR(    69  `} z,Specifics of the emergency-response modeling--,   09  ` jEstimates have to be conservative; Doses are more appropriate characteristics than concentrations (because of their monotonous dependence from the exposure/averaging time); Models should work in two regimes corresponding to potential (emergency response planning) and actual accidents Z H  0޽h ? 33___PPT10i.&gPf+D=' = @B +  0L0 P U(     69  `} TAnalytical approximation of the numerical solution of ADE for a ground-level sourceUUT \  S A ??]o \  S A ??C   ^  6  \  S A ??F l  ^  6j j \   S A ?? '   B8 9   ]are constants.      0  Qwhere 2   c $ "`   This expression is resolved to determine the scale of contamination; The exposure time is 1 hour or more; The governing parameters are the wind speed and direction, and l; in the case of liquid spills, the air temperature is accounted for too; An impact for a ground-level source is considered as a majorant for those for an elevated source; Majorants are calculated for given intervals of U, wind direction and l; Dose criteria are listed for 34 poisonous pollutants. r 2m?J8H0  $   x H  0޽h ? 33___PPT10i.'g5+D=' = @B +~ 0L0 }u (    6\   `} 9Validation of the MGO emergency-response dispersion model::9 "  s * "`z  81  Stable stratifications (Mubareck field test, MGO); 2 - Stable stratifications (Prairie Grass, Green Glow, Ocean Breeze, Dry Gulch  after D. Slade); 3  Neutral stratifications (Prairie Grass, Green Glow, Ocean Breeze, Dry Gulch  after D. Slade); 4 - Unstable stratifications (Prairie Grass, Green Glow, Ocean Breeze, Dry Gulch  after D. Slade); 5 - Neutral stratifications (wind tunnel  after J. Solaile) 2H  p   x  <A H??M [  H6  s *l "` q  `Here D was calculated as a conditional majorant corresponding to given meteorological conditionsa 2a.'  1 H  0޽h ? 33___PPT10i.'glP+D=' = @B +M 0L0 LD D(  D D 6   `} .STATISTICAL FORECASTS IN RUSSIA: STATUS REPORT,/ ".  D s *P  "`]9 <Routine forecasts produced in 235 cities on daily basis in 2002 using statistic models (SMs) developed for each of these cities using the same methodology; Dimensionless parameter P predicted with SMs characterizes unfavorable meteorological conditions that could lead to high levels of air pollution over the whole urban area: P = m/n, where "n" is the total number of measurements during the day and "m" is the number of measurements in excess of 1.5 of corresponding seasonal average values; A quantified characteristic of the synoptic situation is used as a synoptic predictor S; "Previous" value of P is used as a predictor ("inertial factor");@KP PPPHX  l   H D 0޽h ? 33___PPT10i.fO+D=' = @B +  0L0  H0(  Hx H c $ j   x H c $H Pe   H H 0޽h ? 33___PPT10i.f +D=' = @B + 0L0 0T}(  T T 6Xչ   `} y+MAIN STEPS OF TRANSFORMATION OF PREDICTORS,,+ R T 0ع  ]q Normalization of daily maxima (optional): Cmax !B = Cmax / Cseason; Censuring the sample to exclude smallest concentrations (optional; uses P); Transformation of the predictant to the normal distribution; Transformation of nonlinear dependencies in linear ones. * Z0 +      f    9 ^ T 6 T 0(    > 2 H T 0޽h ? 33___PPT10i.f0y+D=' = @B +5 0L0 4,@X(  X X 6   `} v(GENERAL FORMULATION OF THE MODEL IN USE))(  X 0x Y HThe prognostic equation is written as follows: Bt+1 = a0 + ai[Xi] , where [Xi] are transformed predictors Xi at the moment "t", and coefficients "a" are determined using the method of the stepwise regression.  ZZ0" "" """"*"""*"""" " " * " " " * "d " " R;    | QvwH X 0޽h ? 33___PPT10i.fpn+D=' = @B +6 0L0 55PFR`85(  ` ` 64   ` n EFFICIENCY OF TRANSFORMATIONS /1!!  $4t 0 R` #"&mmmmm0 ` 6x ?  j0.57  @` ` 6x ?e  j1.05  @` ` 6x ?r e j0.84  @`  ` 6x ?<  r j1.96  @`  ` 6x ?  <  j2.62  @`  ` 6lx ?  j2.82  @`  ` 6   ?  k2.82   @`  ` 6$  ?j  h70  @` ` 6  ? j Censur.+Norm +Linear"    @` ` 6(  ?0  hd)  @` ` 6  ?9   j0.65  @` ` 6  ?e9   j1.09  @` ` 6p  ?r9 e  j0.78  @` ` 68  ?< 9 r  j1.64  @` ` 6|  ? 9 <   j2.62  @` ` 6\  ?9   j2.77  @` ` 6  ?9   k2.82   @` ` 6  ?j9   h70  @` ` 6  ?9 j  Censur.+ Linear "    @` ` 6y  ?09   hc)  @` ` 6  ?9  j0.91  @` ` 6؍  ?e9  j1.10  @` ` 6  ?re9  j0.58  @` ` 6L  ?< r9  j1.51  @` ` 6 ? < 9  j2.62  @` ` 6 ? 9  j2.82  @`  ` 6 ?9  j2.82  @` !` 6l ?j9  h70  @` "` 6  ?j9  |Censur.   "   @` #` 6tI  ?09  hb)  @` $` 6I  ?_ j1.61  @` %` 6I  ?e_ j1.10  @` &` 6R ?r_e j0.54  @` '` 6 R ?< _r j1.22  @` (` 6 R ? _<  j2.26  @` )` 6R ?_  j1.82  @` *` 6* ?_ j1.82  @` +` 6e ?j_ i160  @` ,` 6» ?_j hNo  @` -` 6T̻ ?0_ ha)  @` .` 6<ֻ ?_ |sm/p(   @` /` 6ϻ ?e_ k  @` 0` 6 ?re_ lCorr  @` 1` 6 ?< r_ xsp(   @` 2` 6  ? < _ zsm(   @` 3` 6 ? _ 2   @`  4` 6p ?_ 2 .    @` 5` 6 ?j_ {Sam-ple"   @` 6` 6 ?j_ Trans-forma-tion"    @` 7` 6 ?0_ kFig"  @`fB 8` 6o ?0`B 9` 01 ?0__`B :` 01 ?0`B ;` 01 ?09 9 `B <` 01 ?0  fB =` 6o ?0fB >` 6o ?00`B ?` 01 ?`B @` 01 ?jj`B A` 01 ?`B B` 01 ?`B C` 01 ?  `B D` 01 ?< < `B E` 01 ?rr`B F` 01 ?ee`B G` 01 ?fB H` 6o ?H ` 0޽h ? 33___PPT10i.fw+D=' = @B +m 0L0 ld` \(  \ \ 6  `} n EFFICIENCY OF TRANSFORMATIONS /2!!  Z \ S \A ?*  Z \ S \A ? Q  Z \ S \A ?S   ^ \ 6  \  \ S A   ?? # <  H \ 0޽h ? 33___PPT10i.f@_+D=' = @B +@ 0L0 ?7pld(  d Id 6, 'g HPERFORMANCE OF STATISTICAL FORECASTS AT INDIVIDUAL MONITORING STATIONSIIH Ut - ld #"&- Kd < ?D ? - $(0.45;14.4), (0.48;16.4), (0.37;9.8)%%$  @` Ld <dҦ ?? D - mBenzene  @` Md <ۦ ?? - kUfa  @` Nd < ?D R ?  %(0.61;22.4), (0.55;26.4), (0.50;20.3)&&%  @` Od < ?R D ?  t Ethylbenzene     @` Pd <ߦ ?R ?  kUfa  @`1 Qd <dc ?D R  W(0.38;11.2), (0.37;10.1), (0.42;9.6), (0.48;11.2), (0.48;10.9), (0.42;9.5), (0.36,17.2)XXW  @` Rd <P ?D R  hHF  @` Sd <ȳ ?R  q Krasnoyarsk     @`= Td <P ?D  c(0.34;7.8), (0.36;14.0), (0.36;10.2), (0.55;30.3), (0.61;22.4), (0.52;21.4), (0.30;7.6), (0.36;9.9)ddc  @` Ud <\ ?D  wCS2&   @` Vd < ? q Krasnoyarsk     @` Wd 6 ?D  (R2; F) at each station.  @` Xd 6< ?D  o Pollutant     @` Yd 6 ? jCity  @`fB Zd 6o ?`B [d 01 ?`B \d 01 ?`B ]d 01 ?R R `B ^d 01 ?? ? fB _d 6o ?--fB `d 6o ?-`B ad 01 ?-`B bd 01 ?D D -fB cd 6o ?-6 dd 0A8,YL jOn average, R2 ~ 0.4  0.6 with independent data sets46(2  (5 H d 0޽h ? 33___PPT10i.f@+D=' = @B + 0L0 hW(  h h 68  `} q#OZONE MONITORING IN ST. PETERSBURG$$# @ h 008  Started in a street canyon in 1998 with two DOAS instruments located at 3 m and 15 m height; several monitors were additionally put in operation last year by the city; The data set in the street canyon is not homogeneous because the pattern of traffic changed several times; Meteorological mast is mounted on the top of the building with DOAS instruments; Concentrations are usually rather moderate. Z H h 0޽h ? 33___PPT10i.f`;+D=' = @B +d< 0L0 c;[;`qvl:(  l l 0h8PP 7SCHEMATIC LAYOUT OF DOAS INSTRUMENTS IN ST. PETERSBURG080( 27 8 M l 0\8p  }Fig. 1. Upper level site 1 - Meteorological mast; 2 - Upper level instruments (emitter, receiver) ; 3 - Upper level mirror.@0 e0  f  ~ d l <̙?@- d l <?P p dR l <?P-@j  l B?  j  l B? p j  l B?   p j  l B? ` K  l jA ? Stationery K l jA ? 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